Schoenebeck Group
@Schoenebeck_Lab
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Last Seen Profiles
A warm welcome to our new colleague Daniele and his team
@LeonoriLab
. We are excited to have you with us in Aachen
@RWTH
.
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8
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PhD position available in our lab to research at the interface of organic synthesis, catalysis and computations. To apply please get in touch with Franziska.
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We are very happy and honored that our chemistry with NMe4SCF3 was selected for 2020 EROS Best Reagent Award. Many thanks to Aldrich® Chemistry, John Wiley & Sons, and the Award Committee.
5
22
253
Have a look at our new air-stable Pd(I) dimer
@angew_chem
. It triggers E-selective olefin migrations in air! It is also a great catalyst for site-selective C-C couplings in air. Congrats Gourab and Theresa!
0
31
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Have a look how unsupervised machine learning with only 5 experimental data points along with in-silico data predicted phosphine ligands (including never made ones) that form air-stable Pd(I) dimers.
@JulianHueffel
@noalasinrazon
@ScienceMagazine
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31
237
Pleased to report a synthetic access to the N-CF3 carbonyl motif in
@Nature
. Interestingly, the N-CF3 amides are more stable than conventional amides, while less conformationally restricted. 95 compounds made. Fantastic work Thomas & Sam!
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With gratitude for the confidence placed in her and a heavy heart to leave
@thiemechemistry
, Franziska is honored to serve the community as part of the editorial team
@J_A_C_S
from 2021.
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6
206
Deeply grateful to be selected for this incredible honor. Many many thanks, especially to my amazing research group – past and present.
🥳We are delighted to announce the winners of the Tetrahedron Young Investigator Awards for 2022. Please join us in congratulating Franziska Schoenebeck
@Schoenebeck_Lab
and Yimon Aye
@EPFL_CHEM_Tweet
! More:
#ChemTwitter
#TetrahedronPrize
#WomenInScience
3
22
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We report trialkylphosphine-derived Ni(I)-dimers & their application, guided by machine-learning. Such ligands are ineffective at displacing COD from Ni(COD)2, offering an alternative access to trialkylphosphine-bound Ni species. Have a look
@J_A_C_S
:
0
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We are looking for a new colleague. All career levels (starting junior academics or more advanced) are welcome to apply. Feel free to reach out for additional information.
0
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Have a look at the triply selective and sequential diversification of a single Csp3 carbon carrying halogen, Bpin and GeEt3 for the modular construction of sp3-rich molecules.
@angew_chem
Congratulations Eric, Markus, Gurdeep, Quentin & Alba!
2
12
188
Happy to share: "Orthogonal Olefination with Organogermanes". Just out
@angew_chem
. Congratulations Amit and Markus.
2
12
174
Happy to report a route to the uncharted chemical space of N-CF2H carbonyl compounds: efficient access to N‑difluoromethyl amides, (thio)carbamates, ureas, formamides & derivatives. Congrats Filip, Gina & Linhao!
@J_A_C_S
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15
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Happy to share an orthogonal C-O coupling of aryl germanes, which tolerates halides, silanes and boronic acid derivatives and proceeds at r.t. under air-tolerant and base-free conditions. Congratulations Amit and Avet.
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161
Happy to share the straightforward and site-selective nitration of aryl germanes at room temperature. Congratulations to Amit, Avet and Aymane (aka the A-team)!
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Have a look at our latest report, featuring remote arylation in less than 10 min reaction time at room temperature enabled by an air-stable Pd(I) dimer
@angew_chem
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For those interested in catalysis with Pd(I) dimers: have a look at our recent minireview
@angew_chem
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One transition state - two different products?! Check out this transmetalation study. A single TS leads to both, cis- and trans-Pd(II) complexes directly. Divergent mechanisms of trifluoromethylation were also uncovered.
#physorg
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137
Happy to share our latest developments to make N-CF3 hydrazines, N-CF3 indoles and their derivatives. All compounds are remarkably robust to acids, bases and further transformations. See
@angew_chem
1
13
122
Happy to share a straightforward route to cyclic and acyclic functional alkyl germanes as part of a special Synthesis issue in celebration of Prof. Cristina Nevado and her 2021 Margaret Faul Award. Congratulations Cristina!
@NevadoLab
@thiemechemistry
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12
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Thank you so much. It was a great conference of which another personal highlight was the chance to interact with so many incredibly enthusiastic young scientists! Great next generation coming up.
A huge congratulations to Franziska Schoenebeck
@Schoenebeck_Lab
on the Tetrahedron Young Investigator Award for Organic Chemistry, here accepting her certificate - the award lecture is up next! 🥳👏
#TETSymp
#award
#WomenInChem
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Happy to share our method to make N-CF3 formamides, just out
@angew_chem
. The N-CF3 formamides are highly robust, compatible with diverse chemical transformations & are conformationally more flexible than e.g. their N-Me analogues. Congrats Filip & Chris!
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We are pleased to report the “Gold-catalyzed Chemoselective Couplings of Polyfluoroarenes with Aryl Germanes and Downstream Diversification”
@J_A_C_S
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Pleased to share Ajoy's, Theresa's and Sinem's work on "E-Olefins through intramolecular radical relocation", published in
@sciencemagazine
.
@RWTH
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Franziska is delighted and looks forward to be the 2021 Streitwieser lecturer
@UCBerkeley
next year in honor of one of the most prominent physical organic chemists, Professor Andrew Streitwieser.
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Germylation of Arenes via Pd(I) Dimer Enabled Sulfonium Salt Functionalization
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Many thanks to the European Research Council for the continued support of our research with a Consolidator Grant. 🇪🇺
📢 Consolidator Grant results! 301 excellent researchers received
#ERCCoG
worth in total €600 million - to address frontier research questions, build up their teams and have far-reaching impact.
🇪🇺
#EUfunded
@EUScienceInnov
@EU_Commission
@GabrielMariya
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On 1st February 2020 our group had its 10 year anniversary. Past and present group members, representing over 20 different nationalities, (re)united for a few days of celebration in the Alps. Diversity has been key to our creativity, innovation and success over the years.
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Pleased to share our latest work: "Orthogonal Stability & Reactivity of Aryl Germanes Enables Rapid and Selective (Multi)Halogenations".
Congratulations Christoph & Kristina.
0
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Happy to report the "Modular & Selective Arylation of Aryl Germanes (C-GeEt3) over C-Bpin, C-SiR3 and C-Halogens enabled by Light-Activated Gold-Catalysis"
@angew_chem
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We are pleased to share the selective and sequential functionalization of C-Br vs. C-Cl vs. C-OSO2F (fluorosulfate). The site-selectivity is independent of any steric or electronic effects imposed by the substrate and fully predictable.
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Although historically aryl germanes were of lower reactivity than other coupling partners, we could recently show their selective and orthogonal functionalizations, outcompeting many established coupling partners. For an overview, please see:
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Chemists randomly running into each other at Kauai’s Waimea Canyon
@WIPOS2023
@ParasramLab
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We very much enjoyed
#ORCHEM22
. Thank you for the organization, great program & also discussions at our posters on our research with organogermanes, Pd(I) catalysis, NCF3 compounds & data science.
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Congratulations Teresa on winning a poster prize at WIPOS 2023
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Pleased to share an alternative use of TMAF for the direct methylation of amides.
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Check out our latest work
@angew_chem
on the mechanism of transmetalation of Pd(II)-F with R3SiCF3. A difluorocarbene is released that then reacts with Pd(II)-F. Congratulations Maoping (
@maoping123
), Italo and Erdem!
#experiments
#computation
#dynamics
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Thank you
@VarinderAggar11
,
@BristolChem
and the 600 attendees for a spectacular 20th Bristol Synthesis Symposium – great science, stimulating discussions and a lot of fun, too!
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Huge thanks to Ilan
@GroupMarek
for being a fantastic host of the 11th Asian-European Symposium. Thanks also to
@anatmilo
@AMSzpilman
@PappoDoron
@AhmadMasarwa2
Gabriel Lemcoff for teaching me on so many fascinating aspects about Israel, including what life in a Kibbutz is like!
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Congratulations to the newly minted Professor Teskey and team! Thanks for having been a great colleague over the years, Chris. We look forward to witnessing Team Teskey's continued success in the years to come.
Delighted to join
@tuBraunschweig
@OCTUBS
from today and looking forward to the exciting times ahead! This follows a fantastic 4.5 years
@RWTH
... I am incredibly grateful to
@Schoenebeck_Lab
for such strong support during this time.
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Had a fantastic time visiting BI, MIT, Boston College & Columbia this week. Many thanks to all and the great honor to be selected as this year's Boehringer-Ingelheim-MIT and Boston College Merck Symposium Lecturer.
@boehringerus
@ChemistryMIT
@Ruck_chem
@TomislavRovis
@j_a_byers
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Check out our latest work
@angew_chem
on polymerization under Pd(I) dimer catalysis: one catalyst, many polymers, within seconds in air.
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For those interested in a compact overview on “Established and Emerging Computational Tools to Study Homogeneous Catalysis - From Quantum Mechanics to Machine Learning”: our article is freely accessible until 25th September.
@Chem_CP
Here is the link:
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Check out our latest
@angew_chem
: ArGeR3 are super robust and the least reactive in Pd(0)/Pd(II) catalysis, yet the most reactive groups with Pd nanoparticles, outcompeting established coupling partners. A molecular mechanism is provided too.
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Many congratulations to our two new PhD graduates: Dr Theresa Sperger and Dr Thomas Scattolin! They are real stars in synthesis, catalysis & computations, having published 20 publications combined (so far).
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It was a pleasure to participate in the 21st CSCB symposium in Dublin. Thank you Pat
@GuiryGroupUCD
for the great hospitality. Also enjoyed the surprise added day of sightseeing (caused by the snowy weather flight chaos).
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Meet our newest lab members. We are happy to welcome Gina, Mathilde and Andrea. All the best for your PhD studies and postdoc.
#InternationalWomensDay
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Check out our latest findings: although ArGeEt3 are lousy coupling partners in Pd(0)/Pd(II) catalysis, they are highly reactive in gold-catalyzed couplings with ArH. Great work Christoph, Amit and Will!
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Check out our latest work on trifluoromethylation
@angew_chem
by our rising Australian star Sinead Keaveney
@Schoenebeck_Lab
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Ending the year on a high note: epic 2023 holiday party!
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We are deeply saddened to have lost our dear colleague, mentor and friend Dieter Enders. Our thoughts are with the Enders Family.
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Future collaboration between AZ and GSK in the making after randomly meeting in a pub in Cambridge...
@NikkiG_Conshy
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Pleased to report the selective arylation and alkylation ortho to an adamantyl group. The oxidative addition to C-Br ortho to the adamantyl group was found to be as favored as to the corresponding adamantyl-free system due to attractive dispersion forces.
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We have some catching up to do on this medium. Check out our recent development to access aryl germanes.
0
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Great collaboration with
@RovisGroup
@TomislavRovis
is now online.
Direct α-alkylation of primary aliphatic amines enabled by CO2 and electrostatics ($)
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Check out our arylation of axially chiral phosphorothioate salts. While Pd(0)/Pd(II) catalysis was found to be ineffective due to a disfavored exchange at Pd(II) and high reductive elimination barrier, Pd(I) catalysis proceeds with favorable driving force.
0
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27
Very happy to see this fantastic work by our two former group members Guoyin Yin and Ignacio Funes-Ardoiz. Many congratulations!
In
@ScienceMagazine
this week, Guoyin Yin’s group uses bulky boron to direct axial substituents onto cyclohexanes that already have an equatorial group
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Deeply honored and humbled to be the recipient of the 2020 Klung-Wilhelmy-Wissenschafts-Preis. A fantastic recognition of the entire team’s efforts over the years – past & present. Thank you so much.
Morgen um 17.30 Uhr wird Prof. Dr. Franziska Schoenebeck von der
@RWTH
mit dem Klung-Wilhelmy-Wissenschafts-Preis für Chemie 2020 ausgezeichnet. Die Anmeldung zur Preisverleihung ist noch bis morgen um 12 Uhr möglich.
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Congratulations to our awesome postdocs Dr. Aymane Selmani and Dr. Adele Queen on their new positions at BASF and Pharmaron UK. A big welcome to our new group member Dr. Lars Gnaegi who is supported by a SNSF postdoctoral fellowship.
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N-CF3 alkynamides & many valuable derivatives, such as N-CF3 decorated alkenyl amides, oxindoles or quinolones - all stable & accessible. Have a look:
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After a too long time apart we were recently finally able to get together again for a climbing activity and to catch up on all the missed celebrations.
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Brilliant! Nice to see you both.
Visit to
@IncParaza
and meeting with former group member Samir of
@Schoenebeck_Lab
(slide of our collaboration with Franziska for effect)
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Happy Birthday
@MarkLautens
and thanks to everyone who already agreed to contribute to this special issue in Mark's honour.
Happy 60th Birthday to our Editor
@MarkLautens
. 🎉👏In his honour, we will publish a special issue on "Domino C-H functionalization reactions and cascade catalysis". ✍️Submissions are welcome❗️For further information contact Franziska Schoenebeck
@Schoenebeck_Lab
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Congratulations to Marvin on the Procter & Gamble prize for his chemistry degree results, a poster prize for his research and a prize by the city of Aachen for volunteer work (Hêvî e.V.) to help students with less priviliged backgrounds. [Marvin pictured in his signature outfit.]
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Our report from earlier this year belongs to the most accessed articles in
@angew_chem
in the period 11/2016 to 10/2017.
Efficient Synthesis of Trifluoromethyl Amines through a Formal Umpolung Strategy from the Bench-... (Schoenebeck)
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The annual New Year's Symposium took place today
@RWTH
. Congratulations to Thomas
@Schoenebeck_Lab
for his poster prize.
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Congratulations to our two new doctors, Sinem and Erdem. Well done!
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A big thank you to the Volkswagen foundation
@VolkswagenSt
in supporting our ideas on "accelerating development with machine learning and data mining". Please apply if you are interested to work with us on this theme.
#Katalyseforschung
: Die
@VolkswagenSt
unterstützt ein Forschungsvorhaben des Arbeitskreises von Prof. Franziska Schoenebeck vom
#RWTH
-Lehrstuhl für Organische
#Chemie
I.:
#DataMining
#MachineLearning
#KI
#AI
#ArtificialIntelligence
#KuenstlicheIntelligenz
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Thomas' work “Efficient Synthesis of Trifluoromethyl Amines through a Formal Umpolung Strategy from the Bench-Stable Precursor (Me4N)SCF3”, published in Angew. Chem., was one of the journal’s top 20 most downloaded recent papers.
#top20article
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Congratulations Chris.
Deeply honoured to have received the ADUC prize for 2022 at the
#Chemiedozententagung
with two other amazing chemists. Many thanks to the board for this recognition and to my fantastic team for their hard work and enthusiasm over the last 3 years.
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Congratulations to our alumnus Dr Thomas Scattolin who was selected as a
@Reaxys
finalist for his work on developing an efficient route to trifluoromethyl amines, published in
@angew_chem
.
#ReaxysPhDPrize
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Dining in style with great company
@HartungIngo
@Bayer
. Looking forward to an exciting day tomorrow
@Bayer
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Have a look also at our recent Ni-catalyzed remote functionalization of ketones.
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Many congratulations to Indrek Kalvet for winning a major research award in the Estonian student research contest. Picture shows Indrek at the award ceremony at the Estonian ministry of research.
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Cakes at group meeting today on the occasion of Indrek's thesis submission and to welcome visitor Yuuta from Kyoto and apprentice Mike!
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Claudia and Christoph from
@Schoenebeck_Lab
had a blast at
#omcos20
- great science, discussions and venue! Thank you to the organizers.
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Fantastic to see Ignacio being recognised for his great work. Many congratulations. Very happy for you.
Happy to get this wonderful recognition from Suschem Spain. The platform highlights the last project I was involved in the
@Schoenebeck_Lab
about unsupervised machine learning applied to Pd chemistry. Thanks Franziska and
@AvHStiftung
for the nice stay in Germany!
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Join us for the upcoming special topics issue on halogenation methods (with a view towards radioimaging applications) in Synthesis
@thiemechemistry
. Submissions are welcome.
Interested in the structural behaviour of Willgerodt-type Dichloro(aryl)-λ3-Iodanes? Check out our latest paper as part of the Synthesis special edition on halogenation! Congratulations Jérôme and Jessica!
@WWU_Muenster
@thiemechemistry
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@JulianHueffel
@noalasinrazon
@ScienceMagazine
Many congratulations to Julian (
@JulianHueffel
), Theresa, Ignacio (
@noalasinrazon
) and our collaborators Yas and Kari.
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Opportunities for Master and PhD studies at the Max Planck School Matter to Life. Apply under:
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Super news! Many congratulations. We all look forward to having you on the team.
So ecstatic to have received this award! Many thanks to the
@GDCh_aktuell
and
@clariant
for the support. Can't wait to start my postdoc position with the
@Schoenebeck_Lab
this summer!
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Happy Birthday
@houk1000
Awesome dinner with the incomparable Ken Houk, Ged Parkin and
@SoyLuisCampos
Happy birthday, Ken!
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Ignacio Funes now leads his own research group at the University of La Rioja in Spain. Congratulations.
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@ThomasScattolin
, our group's alumnus and N-CF3 pioneer, now excelling at Mirati in San Diego, is a recipient of the 2023 Industrial Early Career Investigator Award! Many congratulations. We are looking forward to your lecture at the ACS.
Next up: Congratulations to the
@ACSorganic
2023 Industrial Early Career Investigator Awardees! Looking forward to an amazing set of award talks in San Francisco!
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@TheCycloEdition
@angew_chem
We really enjoyed this episode. Great job! Well done and many thanks.
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Thanks for the warm welcome. 😊
Let’s welcome the Schoenebeck Group to Twitter! We’ll look forward to seeing announcements of their groundbreaking Pd- and Ni-mediated transformations
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@funes_ardoiz
@MaserasGroup
@Diego__Sampedro
@unirioja
Brilliant news. Many congratulations Ignacio!!
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